Vision
The technical vision of our project is the development of a
continuous, wearable progesterone monitor. Our team has sided with using
bio-impedance based aptasensors as the current means of achieving this
goal (see science section below). Our interest in aptamers is due to
their modular nature, expanding user base, versatility, safety,
simplicity, and low entry cost1.
This technology has several potential applications, due to progesterone
levels’ time-dependent variability2
and their link to female health, including the fertility window3, menopause4 and women’s cancer5. Our team is focused on using this
technology to illuminate early pregnancy and miscarriage, which has
historically been shrouded in stigma (see home page) and continues to
harbor important knowledge gaps6.
Miscarriage is relatively common, with approximately 1 million
pregnancies per year ending in miscarriage in the United States6. Although about half of these
miscarriages are due to well-understood genetic abnormalities7, a significant portion of the remaining
miscarriages are not well understood6,8. As a key, variable female sex hormone
involved in pregnancy and miscarriage3,5,9, progesterone is poised to provide
additional insights into miscarriages when monitored at sufficient
frequency and accuracy. Currently, progesterone is monitored through
blood draws or urine tests10, which
limits the regularity, frequency, and ease with which these tests can be
administered3. Developing a
continuous progesterone monitor would add a new dimension to women’s
health research, allowing for improved research in women’s health and
miscarriage.
Some specific potential outcomes are a better picture of individual
and chronological variability of progesterone levels during early
pregnancy, a better understanding of the chronological link between
progesterone levels and miscarriage, and leading miscarriage prediction,
detection and classification capabilities. Providing these capabilities
directly to women rather than through a medical provider is valuable.
More information will create more advocacy for women to allow women to
take ownership of their own health. Through our interviews and online
research, we have found that women often are not seen by medical
providers until 10 weeks into their pregnancy11, by which point many miscarriages will
already have occurred12, possibly
without their awareness13. Studies
have shown that the blood concentration of progesterone is related to
the rate of miscarriage14. By
creating a wearable continuous progesterone monitor, we hope to
continuously monitor precise levels of progesterone to inform pregnant
women on the health of their pregnancies. Although our tool alone is not
enough to completely demystify the phenomenon or to remove the
historical stigma surrounding it, we believe it will
- provide researchers with a new dimension of data collection,
facilitating novel research in the areas of early pregnancy and
miscarriage
- provide women with information, education, and a means of
self-monitoring, self-advocacy, and empowerment during early pregnancy
and miscarriage
- serve to drive additional advances in women’s health research and
technology
Although we didn’t begin the year with these aspirations (see our
Journey section below), we feel the problem is a natural fit and aligns
well with the unique aspects of our team. We are students at Brigham
Young University, part of the educational system of The Church of Jesus
Christ of Latter-day Saints. The Church and we as members deeply value
the ability of couples who so desire to participate in the sacred
process of procreation and childbirth and to start healthy, happy
families15. Many women,
locally16 and globally17, want to have families, but forces
outside of their control such as fertility problems or repeated
miscarriage delay biological childbirth or put it out of reach entirely,
resulting in profound emotional pain. We want to help in some small way
to end that pain. We see this project as a means to help these and other
women create the families they desire.
Science
Early in the year, we decided on aptamer-based detection as our
method of choice, due to its versatility, cost-effectiveness, and
cell-free nature. Based on our conversations with an aptamer expert and
our PI, we felt that an important step in our progress towards building
an aptasensor was our independent validation of the aptamer’s binding
affinity (KD) with the
desired target. This validation would provide us with experience in
confidence that our aptamer was sensitive and specific enough to be
useful in an aptasensor, and provide us with needed lab experience,
given that aptamers are not frequently utilized at BYU and are not an
area of expertise for our PI, Jared Barrott. Prioritizing validation led
us to perform a fluorophore-quencher affinity assay with our selected
PFOA aptamer (PFOA_JYP_2)18, and
later, after a pivot in our population of interest and target molecule,
to validate our selected progesterone aptamer (P4G03)19’s binding affinity. Due to this
aptamer’s different mode of activity (bio-impedance instead of
fluorescence) we chose to validate KD and confirm
conformational change through isothermal titration calorimetry and
circular dichroism.
Simultaneously, we have worked to develop necessary technical
components and expertise to facilitate the development of actual
aptasensors using these sequences. When focused on the fluorescent PFOA
aptamer system, we developed a working fluorescent monitoring system and
custom microfluidic chip to measure environmental concentrations of
PFOA. Once we transitioned to the bio-impedimetric progesterone aptamer
system, we shifted focus to the use of gold electrodes and AC
voltammetry to measure the progesterone induced voltage changes.
Obtaining this aptamer with required electrochemical modifications was
time consuming, so our time for experimentation was limited, but after
three experiments, we have been able to witness electrical signals due
to high concentrations of progesterone using AC voltammetry. We are
currently troubleshooting the chemical procedures for attachment to the
electrode and the use of our specific hardware setup in order to
optimize our signal to noise ratio and to keep the aptamer active on the
electrode surface for as long as possible.
Journey
As part of the Crocker Innovation Fellowship at Brigham Young
University, our team was given the goal to create an Internet of Things
(IOT) device that would be scalable and marketable while meeting the
deeply felt needs of an under-served population. We were taught starting
in January 2025 that picking an initial population to investigate, and
getting to know their needs, pains, and day-to-day inconveniences can
often lead the curious listener to a problem worth solving.
(Visual)
Many of our team members have family or acquaintances that are
firefighters, in either urban or wildland settings, so we began
investigating their experiences through internet research and interviews
with firefighters, chiefs, and researchers to see what pains we could
address. Outside of the immediate danger of getting burned, the
long-term consequences of firefighting we discovered involved greatly
amplified cancer risk due to environmental toxicity. Firefighters have
the highest rate of death from cancer than any other groups in part
because of their constant exposure of PFOA contained in smoke. In
February, we decided to address this issue by creating a device that
would serve as a continuous monitor of airborne PFOA (a specific
carcinogen impacting firefighters) levels. Aptamers were decided on as
the ideal biosensor to address this problem due to their cell-free
nature, versatility, cost effectiveness, and continuous monitoring
capabilities.
During our research and development on our carcinogen biosensor and
our additional human practices research (see human practices page), we
began to sense a need to pivot. We observed that although firefighters
were aware of and in many cases stressed about the risk of developing
cancer, many of the firefighters we interviewed did not value routine
cleaning procedures and other prescribed safety practices designed to
reduce this risk enough to fully comply. Some of our team were
frustrated that firefighters seemed to be more interested in measuring
their personal hormones than carcinogens.
We faced technical uncertainty on the best way to measure cumulative
carcinogen exposure using aptamers in a way that would be both
comprehensive and hassle-free. We also identified competitors - a 2023
iGEM team (FluoroLoop, DTU-Denmark) had used aptamers to detect
PFOA20, and another independent
researcher had found an abiotic method for airborne PFOA measurement
that would likely render our product obsolete. As entrepreneurship in
under-served spaces is an important part of the Crocker Innovation
Fellowship, we felt it was appropriate to pivot.
For a while, we explored the idea of using synthetic biology to
continuously measure heavy metal levels in groundwater. This would help
large, corporate mines in the United States to comply with federal
monitoring regulations. However, we found that our abiotic
competitors21,22 were too advanced,
and although biological sensors had some advantages such as potentially
small size and portability, making a dent in the industry using
synthetic biology would require a larger investment in research and
development than we could afford. After intense discussion and several
presentations from team members on prospective research avenues, we
found progesterone monitoring for the purpose of miscarriage detection
to be a compelling problem, under-served population, and relatively
feasible research direction.
Although we still face technical uncertainty and have identified
adjacent technologies that could represent competitors (Ava23 and Mira24), we feel that our solution would
provide a technical edge through direct and continuous progesterone
monitoring, something not seen currently on the market. Additionally, we
have identified target research grants and other sources of investment
that might allow us to surpass our current technical limitations through
the acquisition of new resources, tools, perspectives, and
experience.
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